Common glass-forming spin-liquid state in the pyrochlore magnets Dy2Ti2O7 and Ho2Ti2O7

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dc.contributor.author Eyvazov, Azar B.
dc.contributor.author Dusad, Ritika
dc.contributor.author Munsie, Timothy J. S.
dc.contributor.author Dabkowska, Hanna A.
dc.contributor.author Luke, Graeme M.
dc.contributor.author Kassner, Ethan R.
dc.contributor.author Davis, J. C. Seamus
dc.contributor.author Eyal, Anna
dc.date.accessioned 2019-04-10T15:47:15Z
dc.date.available 2019-04-10T15:47:15Z
dc.date.issued 2018-12-18
dc.identifier.citation Eyvazov, A. B., Dusad, R., Munsie, T. J. S., Dabkowska, H. A., Luke, G. M., Kassner, E. R., Davis, J. C. S. and Eyal, A. (2018) ' Common glass-forming spin-liquid state in the pyrochlore magnets Dy2Ti2O7 and Ho2Ti2O7’, Physical Review B, 98 (21), 214430 (9 pp). doi: 10.1103/PhysRevB.98.214430 en
dc.identifier.startpage 1 en
dc.identifier.endpage 9 en
dc.identifier.issn 2469-9950
dc.identifier.uri http://hdl.handle.net/10468/7750
dc.identifier.doi 10.1103/PhysRevB.98.214430 en
dc.description.abstract Despite a well-ordered pyrochlore crystal structure and strong magnetic interactions between the Dy3+ or Ho3+ ions, no long-range magnetic order has been detected in the pyrochlore titanates Ho2Ti2O7 and Dy2Ti2O7. To explore the actual magnetic phase formed by cooling these materials, we measure their magnetization dynamics using toroidal, boundary-free magnetization transport techniques. We find that the dynamical magnetic susceptibility of both compounds has the same distinctive phenomenology, which is indistinguishable in form from that of the dielectric permittivity of dipolar glass-forming liquids. Moreover, Ho2Ti2O7 and Dy2Ti2O7 both exhibit microscopic magnetic relaxation times that increase along the super-Arrhenius trajectories analogous to those observed in glass-forming dipolar liquids. Thus, upon cooling below about 2 K, Dy2Ti2O7 and Ho2Ti2O7 both appear to enter the same magnetic state exhibiting the characteristics of a glass-forming spin liquid. en
dc.description.sponsorship Gordon and Betty Moore Foundation (Moore Foundation's EPiQS Initiative through Grant No. GBMF4544) en
dc.format.mimetype application/pdf en
dc.language.iso en en
dc.publisher American Physical Society en
dc.relation.uri https://link.aps.org/doi/10.1103/PhysRevB.98.214430
dc.rights © 2018 American Physical Society en
dc.subject Spin ice en
dc.subject Spin liquid en
dc.subject Glassy systems en
dc.subject Magnetic systems en
dc.subject Artifical spin en
dc.title Common glass-forming spin-liquid state in the pyrochlore magnets Dy2Ti2O7 and Ho2Ti2O7 en
dc.type Article (peer-reviewed) en
dc.internal.authorcontactother J. Seamus Davis, Physics, University College Cork, Cork, Ireland. T: +353-21-490-3000 en
dc.internal.availability Full text available en
dc.description.version Published Version en
dc.contributor.funder Gordon and Betty Moore Foundation en
dc.description.status Peer reviewed en
dc.internal.IRISemailaddress james.davis@ucc.ie en
dc.identifier.articleid 214430 en
dc.identifier.eissn 2469-9969


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