Isotropic and anisotropic collision-induced Raman scattering by monoatomic gas mixtures: Ne-Ar
dc.contributor.author | Dixneuf, Sophie | |
dc.contributor.author | Chrysos, M. | |
dc.contributor.author | Rachet, F. | |
dc.date.accessioned | 2017-08-25T10:08:52Z | |
dc.date.available | 2017-08-25T10:08:52Z | |
dc.date.issued | 2009 | |
dc.description.abstract | We report the long-overdue collision-induced Raman scattering spectrum by a pair of unlike rare gas atoms. Absolute-unit scattering intensities, both isotropic and anisotropic, are given for Ne-Ar, along with the depolarization ratio for this system, recorded by a gaseous room-temperature mixture over a wide range of frequency shift. We make a critical comparison with spectra computed quantum-mechanically on the basis of modern pair-polarizability representations for Ne-Ar, of either ab initio or density functional theory methods. We report a value for the Kerr second virial coefficient, deduced from our measurements. Our data are especially intended to add to the vital yet hitherto incomplete knowledge of the role of collision-induced processes in atmospheric environments. | en |
dc.description.status | Peer reviewed | en |
dc.description.version | Published Version | en |
dc.format.mimetype | application/pdf | en |
dc.identifier.articleid | 22703 | |
dc.identifier.citation | Dixneuf, S., Chrysos, M. and Rachet, F. (2009) 'Isotropic and anisotropic collision-induced Raman scattering by monoatomic gas mixtures: Ne-Ar', Physical Review A, 80(2), 022703. (8pp). doi: 10.1103/PhysRevA.80.022703 | en |
dc.identifier.doi | 10.1103/PhysRevA.80.022703 | |
dc.identifier.issn | 1050-2947 | |
dc.identifier.issn | 1094-1622 | |
dc.identifier.issued | 2 | |
dc.identifier.journaltitle | Physical Review A | en |
dc.identifier.uri | https://hdl.handle.net/10468/4533 | |
dc.identifier.volume | 80 | |
dc.language.iso | en | en |
dc.publisher | American Physical Society | en |
dc.relation.uri | https://journals.aps.org/pra/abstract/10.1103/PhysRevA.80.022703 | |
dc.rights | © 2009, American Physical Society | en |
dc.subject | Induced light scattering | en |
dc.subject | Ab initio calculation | en |
dc.subject | Correlated molecular calculations | en |
dc.subject | 2nd virial coefficients | en |
dc.subject | Electric properties | en |
dc.subject | Rare gases | en |
dc.subject | Argon | en |
dc.title | Isotropic and anisotropic collision-induced Raman scattering by monoatomic gas mixtures: Ne-Ar | en |
dc.type | Article (peer-reviewed) | en |
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