Electrofuels in a circular economy: A systems approach towards net zero

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dc.contributor.authorRusmanis, Davisen
dc.contributor.authorYang, Yanen
dc.contributor.authorLong, Aoifeen
dc.contributor.authorGray, Nathanen
dc.contributor.authorMartins, Kelvin C.en
dc.contributor.authorÓ Loideáin, Seán Ógen
dc.contributor.authorLin, Richenen
dc.contributor.authorKang, Xihuien
dc.contributor.authorCusack, Donal Ógen
dc.contributor.authorCarton, James G.en
dc.contributor.authorMonaghan, Roryen
dc.contributor.authorMurphy, Jerry D.en
dc.contributor.authorWall, David M.en
dc.contributor.funderScience Foundation Irelanden
dc.date.accessioned2023-08-02T15:53:19Z
dc.date.available2023-08-02T15:53:19Z
dc.date.issued2023-07-05en
dc.description.abstractDecarbonising the hard-to-abate sectors will be necessary in realising a future net-zero economy. Electrofuels store electricity as low carbon energy vectors such as hydrogen or methane which can be used in areas where electrification is not ideal, and as such can facilitate decarbonisation of sectors such as transport, agriculture, and wastewater treatment. In this study, the production of electrofuels was analysed at an industrial site by storing renewable electricity as green hydrogen produced using electrolysis. The analysis highlighted the need for scale in hydrogen production. The cost of hydrogen was calculated at €8.92/kg when a 122 kW electrolyser operated solely on curtailed electricity generated from the industry site was situated at a 65,000 person equivalent municipal wastewater treatment plant. A subsequent integrated and circular approach to electrofuels production was investigated. The oxygen by-product from electrolysis could be utilised for wastewater aeration and reduce the annual electricity usage at the wastewater treatment plant by 3.6%. Furthermore, the carbon dioxide in biogas generated from sewage sludge could be converted to methane through a Sabatier reaction (4H2 + CO2 → CH4 + 2H2O) as a means of carbon capture and utilisation. The hydrogen produced from the 122 kW electrolyser could convert only 40% of the total carbon dioxide (within the biogas) in a biomethanation process, again supporting the argument for larger electrolyser systems with increased hydrogen production. Pyrolysis of digestate to produce biochar was investigated as a negative emissions technology. If pyrolysis is coupled with anaerobic digestion of feedstocks within 10 km of the industry site savings of 42.7 kt CO2/a could be achieved. In essence, a circular economy approach to electrofuel production could integrate existing electrical, gas and water infrastructure, whilst treating waste, improving the environment, decarbonising agriculture, and storing energy in the form of new low carbon energy vectors for use in heavy transport. Such an approach is vital to progressing future net-zero strategies, however future emissions accountancy processes must adapt to facilitate the benefits of a circular economy.en
dc.description.statusPeer revieweden
dc.description.versionPublished Versionen
dc.format.mimetypeapplication/pdfen
dc.identifier.articleid117367en
dc.identifier.citationRusmanis, D., Yang, Y., Long, A., Gray, N., Martins, K. C., Ó Loideáin, S.Ó., Lin, R., Kang, X., Cusack, D. Ó., Carton, J. G., Monaghan, R., Murphy, J. D. and Wall, D. M. (2023) 'Electrofuels in a circular economy: A systems approach towards net zero', Energy Conversion and Management, 292, 117367 (13pp). doi: 10.1016/j.enconman.2023.117367en
dc.identifier.doi10.1016/j.enconman.2023.117367en
dc.identifier.endpage13en
dc.identifier.issn0196-8904en
dc.identifier.journaltitleEnergy Conversion and Managementen
dc.identifier.startpage1en
dc.identifier.urihttps://hdl.handle.net/10468/14787
dc.identifier.volume292en
dc.language.isoenen
dc.publisherElsevier Ltd.en
dc.relation.ispartofEnergy Conversion and Managementen
dc.relation.projectinfo:eu-repo/grantAgreement/SFI/SFI Future Innovator Prize::Zero Emissions Challenge/19/FIP/ZE/7565/IE/ElectroFuels in A Circular Economy (EFACE)/en
dc.relation.projectinfo:eu-repo/grantAgreement/SFI/SFI Research Centres Programme::Phase 2/12/RC/2302_P2/IE/MAREI_Phase 2/en
dc.rights© 2023, the Authors. Published by Elsevier Ltd. This is an open access article under the CC BY license (http://creativecommons.org/licenses/by/4.0/).en
dc.rights.urihttps://creativecommons.org/licenses/by/4.0/en
dc.subjectElectrofuelsen
dc.subjectGreen hydrogenen
dc.subjectBiomethanationen
dc.subjectCircular economyen
dc.subjectDecarbonisationen
dc.subject~Civil and Environmental Engineering - Journal articles~en
dc.titleElectrofuels in a circular economy: A systems approach towards net zeroen
dc.typeArticle (peer-reviewed)en
oaire.citation.volume292en
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